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Hiraoka K, Sagano W, Nose T, Finkelmann H 2005 Biaxial shape memory effect exhibited by monodomain chiral smectic C elastomers Macromolecules 38:7352 7357 Hogan PM, Tajbakhsh AR, Terentjev EM 2002 UV manipulation of order and macro scopic shape in nematic elastomers Phys Rev E 65:041720 Holland NB, Hugel T, Neuert G, Cattani Scholz A, Renner C, Oesterhelt D, Moroder L, Seitz M, Gaub HE 2003 Single molecule force spectroscopy of azobenzene polymers: switching elasticity of single photochromic macromolecules Macromolecules 36:2015 2023 Hosono N, Furukawa H, Masubuchi Y, Watanabe T, Horie K 2007 Photochemical control of network structure in gels and photo induced changes in their viscoelastic properties Colloids Surf B Biointerfaces 56:285 289 Hu Z, Zhang X, Li Y 1995 Monitoring release of neurotrophic activity in the brains of awake rats Science 269:525 553 Hugel T, Holland NB, Cattani A, Moroder L, Seitz M, Gaub HE 2002.

Fig. 5.45 Single-sweep voltammogram of oxidation of methanol in 0.5 M H2SO4, with the same electrode and the same conditions of methanol adsorption as in Fig. 5.43. Concentrations of methanol (mol dm"3): (1) 0, (2) 10"4, (3) 10-*, (4) 10~2, (5) HT1. (By courtesy of J. Weber)

Red Hat Enterprise Linux 2.1 (update 6) Red Hat Enterprise Linux 3 (update 6) Red Hat Enterprise Linux 4 Novell s SUSE Linux Enterprise Server 9

Single molecule optomechanical cycle Science 296:1103 1106 Ikeda T 2001 Photochemical modulation of refractive index by means of photosensitive liquid crystals Mol Cryst Liq Cryst 364:187 197 Ikeda T 2003 Photomodulation of liquid crystal orientations for photonic applications J Mater Chem 13:2037 2057 Ikeda T, Tsutsumi O 1995 Optical switching and image storage by means of azobenzene liquid crystal lms Science 268:1873 1875 Ikeda T, Horiuchi S, Karanjit DB, Kurihara S, Tazuke S 1988 Photochemical image storage in polymer liquid crystals Chem Lett 17:1679 1682 Ikeda T, Horiuchi S, Karanjit DB, Kurihara S, Tazuke S 1990a Photochemically induced isothermal phase transition in polymer liquid crystals with mesogenic phenyl benzoate side chains 1 Calorimetric studies and order parameters Macromolecules 23:36 42 Ikeda T, Horiuchi S, Karanjit DB, Kurihara S, Tazuke S 1990b Photochemically induced isothermal phase transition in polymer liquid crystals with mesogenic phenyl benzoate side chains 2.

366 or is the result of some other type of inhibition. The steric effect where the sufficiently close approach of the electroactive substance to the electrode is inhibited is typical for large surface-active molecules. The adsorbed layer of surfactant replacing the layer of water molecules covering the surface of the electrode prevents the reacting species and their solvation shells from forming a configuration suitable for the electrode reaction (see Section 5.3). This leads to a decrease in the value of the rate constant of the electrode reaction. For example, in the case of an irreversible electrode reaction with a rate constant kc and adsorption of an uncharged surfactant, we have fcc = fc0(l-O) + fc1 (5.7.18)

where k0 and kY are the rate constants for the electrode reaction at unoccupied and occupied sites of the electrode surface, respectively. For the adsorption of surface-active ions, these quantities are also a function of the surface coverage 0. It is very simple to determine the value of 0 = F/F m for a strongly adsorbed substance in electrolysis with a dropping mercury electrode. If a much smaller amount of substance is sufficient for complete electrode coverage than available in the test solution, then the surface concentration of the surface-active substance F is determined by its diffusion to the electrode. The total amount M adsorbed on the electrode in time t (A is the surface of the electrode according to Eq. (4.4.4) and F is the surface excess in moles per square centimetre) is given as

Photochemically induced isothermal phase transition behaviors Macro molecules 23:42 48..

Standard distributions:

M = 0.85Fm2/V/3 =

Ikeda T, Horiuchi S, Karanjit DB, Kurihara S, Tazuke S 1990c Photochemically induced isothermal phase transition in polymer liquid crystals with mesogenic cyanobiphenyl side chains Macromolecules 23:3938 3943 Ikeda T, Sasaki T, Kim HB 1991 Intrinsic response of polymer liquid crystals in photochemical phase transition J Phys Chem 95:509 511 Ikeda T, Sasaki T, Ichimura K 1993 Photochemical switching of polarizationin ferro electric liquid crystal lms Nature 361:428 430 Ikeda T, Nakano M, Yu Y, Tsutsumi O, Kanazawa A 2003 Anisotropic bending and unbending behavior of azobenzene liquid crystalline gels by light exposure Adv Mater 15:201 205 Irie M 1986 Photoresponsive polymer Reversible bending of rod shaped acrylamide gels in an electric eld Macromolecules 19:2890 2892 Irie M 1990 Photoresponsive polymers Adv Polym Sci 94:27 67 Irie M, Kungwatchakun D 1995 Photoresponsive polymer Mechanochemistry of poly acrylamide gels having triphenylmethane leuco derivatives Makromol Chem Rapid Commun 5:829 832.

(5.7.19)

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