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A different supramolecular approach has been successfully used to design azobenzene-containing materials capable of very effective SRG formation (Kulikovska et al, 2007; Stumpe et al, 2006a) The materials consist of ionic complexes of polyelectrolytes and oppositely charged azobenzene derivatives as counter ions Fig 22 explains schematically the material structures in comparison to the conventional azobenzene-containing materials reported for SRG inscription For the rst time, a very effective light-induced mass transport even superior to that in the functionalized polymers has been demonstrated in the systems, where the chromophores are attached to the passive polymer chains by the noncovalent interactions SRGs with the surface modulation depth up to 165 mm have been obtained using these materials.

IBM has been a leader in the blade market for a variety of reasons. As a leader in the traditional server market and an early entrant in the blade market, IBM offered early adopters an easy decision to migrate from IBM rack servers to IBM blades. With a strong history of backward- and forward-compatibility (as exemplified by compatibility from the original chassis through BladeCenter H), IBM offers a way to implement a wide variety of blade choices, with the low-risk comfort factor of choosing IBM as a long-term blade foundation. Although IBM may not always be the first vendor to offer products with the latest technology, they continue to deliver reliable products which, if not first, follow closely enough thereafter. Finally, the BladeCenter ecosystem continues

to the cathodic electrode reaction. The overall current density is given by the relationship ) = / a +/c = nF(kacRed - kccOx) (5.2.13)

Formation of such deep relief structures evidences that alternatively to covalent bonding, the ionic interactions keep the chains of passive polymer linked to the chromophores, strongly enough to be involved into the light-induced motion of chromophores Since the interactions between azobenzene moiety and a polymer matrix became of particular importance in this latter case of the light-induced mass transport, a few studies on noncovalent intermolecular interactions that have been widely exploited in supramolecular chemistry are discussed They were used, for example, to prepare self-assembled materials (Meier and Schubert, 2005; Pollino and Weck, 2005; Faul and Antonetti, 2003; Ikkala and ten Brinke, 2002) A number of polyelectrolyte surfactant complexes that form lms with low surface energies have been reported (Thunemann et al, 2000, 1999; Antonietti et al, 1994).

In the absence of current (/ = 0), the system is in equilibrium but the electrode reactions nonetheless proceed. Thus, similar to chemical equilibria, the electrode equilibria have a dynamic character. Under equilibrium conditions (5.2.14) Substitution of Eqs (5.2.8), (5.2.9) and (5.2.10) into this equation yields

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The majority of investigations have dealt with dye dye intermolecular interactions, but less effort has been directed toward the study of noncovalent interactions between the active molecules and host material The effect of electronic properties of the host polymer and speci c chromophore host interactions on the electro-optic coef cient of doped polymer lms has been investigated in Banach et al (1999) Recently, the in uence of noncovalent interactions between dye molecules and host polymer on the aggregation tendency of the guest (dye) molecules has been studied (Priimagi et al, 2007, 2006, 2005) The effect of polyelectrolyte matrix on the lm properties has been investigated as well (Meyer et al, 1991; Simmrock et al, 1989) The new materials under discussion have polymerlike properties and thus can be processed from solution to form lms with excellent optical quality and transmission in the visible spectral range.

and, after rearrangement,

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Generally, the polyelectrolyte as a polymer matrix determines the mechanical, thermal, and morphological properties of the system For example, the presence of exible chain segments or a certain amount of irregularity along the polymeric structure reduces recrystallization tendency and improves the stability of the glassy state (Meyer et al, 1991; Simmrock et al, 1989) By these means the thermal behavior and processability of the materials can be in uenced The authors demonstrated variation of the glass transition temperature from 221C to 1911C just by change of organic moieties in either main- or side chains of polyelectrolyte (Simmrock et al, 1989) Also, the charge density and the pH value can affect the structures and the surface energies as it has been shown for the polyelectrolyte surfactant complexes (Faul and.

l ~ R T )

(5215)