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Photoorientation concerns closeorder motion of azobenzene chromophore (rotation), whereas the formation of SRG involves long-distance movement (mass transport) of chromophores and, possibly, of nonphotoactive polymer chains According to Zucolotto et al (2003), the electrostatic interactions between active and inert layers serve as a mean for the SRG formation but, on the contrary, tend to hinder the photoisomerization of azobenzenes This inherent con ict together with restriction of molecules freedom by layered structure explains rather ineffective SRG inscription in LbL architectures The materials used for recording of SRG were similar and are depicted in the Figs 27 and 28 Between them, three azodyes, Direct Red 80, Congo Red, and Brilliant Yellow (Fig 27), were employed For PDADMAC/(Congo Red) structures (He et al, 2000), the dependence of SRG ef ciency on the number of layers was investigated.

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In more complicated reactions, the reaction orders v / a and v, c need not and often do not correspond to the stoichiometric coefficients vir and vio. In contrast to the latter, the reaction orders can often be fractional or even negative. The concentration of a given reactant can sometimes appear in the expressions for both the anodic and the cathodic reaction rates. If it is known which of the reactions determine the rate of the overall complex electrode process, then the concept of the stoichiometric number of the electrode process v is often introduced. This number is equal to the number of identical partial reactions required to realize the overall electrode process, as written in an equation of type (5.2.2).t If the rate constant of this partial rate-determining reaction is /ca, then ka k'Jv. Thus, for example, if the first of reactions (5.1.7) is the rate-determining step in the overall electrode process (5.1.4) then the stoichiometric number has the value v = 2. 5.2.2 The phenomenological theory of the electrode reaction

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Maximum relief height of 140 nm at corresponding rstorder DE of 17% has been achieved for 2-mm thick lm consisting of 640 layers This is actually the highest value reported so far for LbL layers Dependence of the achieved relief height on the number of bilayers is shown in Fig 213 As the lm thickness is of comparable value, used generally for polymer materials, low ef ciency cannot be attributed to layer thickness Also, writing kinetics for thick layers was rather slow at the irradiation intensity of 150 mW/cm2, the maximum of rst-order DE was achieved in 75 min..

As the generality of equations of type (5.2.3) should not be exaggerated (e.g. in the presence of strong adsorption, such as in electrocatalytic processes, they are no longer valid), the basic features of electrochemical kinetics will be explained by using the simple electrode reaction Red<^Ox + Ae z (5.2.5)

The BladeCenter architecture supports up to 14 server blades per chassis, (chassis range from 7U to 9U for BladeCenter and BladeCenter H) and utilizes a passive midplane. Server blades and hot-swappable, redundant loadbalancing power supplies are inserted into the front of the chassis. Shared hotswap, redundant switch modules, management modules, and blowers are inserted in the back. On-blade storage is available, as is shared storage through NAS or SAN. Switch modules are available for GbE, 4 Gig Fibre Channel, 1x InfiniBand, Myrinet, and 4x InfiniBand. Bridges and gateways are available for IB to FC and Ethernet. Blade networking options include additional GbE or 10GbE NICs, iSCSI software initiator for boot from SAN, Fibre Channel HBA daughter cards, and InfiniBand HCAs. Standard Ethernet and Fibre Channel implementations require networking adapters on each blade, which connect to the appropriate switch module in the chassis. Virtualized I/O is available through the IB implementation, with gateways and bridges to connect to non-IB devices. Future plans in this area for Fibre Channel include N-port identifier virtualization (NPIV), which will allow sharing of adapters so that the 14 blades share access to 6 HBAs.

t A different formulation would be: the stoichiometric number gives the number of identical activated complexes formed and destroyed in the completion of the overall reaction as formulated with charge number n.

Figure 2.13. Dependence of surface modulation amplitude (according to AFM measurements) on the number of deposited bilayers in PDADMAC/(Congo Red) LbL lms. Source: He et al., 2000. Reprinted with permission from American Chemical Society.

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