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The electrode reaction occurs in the region where by the influence of the electrode charge an electric field is formed, characterized by the distribution of the electric potential as a function of the distance from the electrode surface (see Section 4.3). This electric field affects the concentrations of the reacting substances and also the activation energy of the electrode reaction, expressed by the quantities wr and wp in Eq. (5.3.13). This effect can be

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This had two purposes: the first was to enable collaborative work through file sharing, and the second was to centralize data onto one server system for ease of file-management tasks (backup, recovery, etc) The leader in this file-server movement was Novell, which at its peak owned 70% of the PC network market At the same time, Sun Microsystems had developed a new protocol called Network File System (NFS) that allowed file sharing across multiple systems Sun released the protocol and a reference port into the public domain in the mid 1980s These file server technologies became the basis for future networked storage, and today nearly all network-attached storage (NAS) implementations are based on NFS or the Microsoft version SMB/CIFS (Server Message Block/Common Internet File System).

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Living systems respond to external stimuli by adapting themselves to changing conditions. Polymer scientists have been trying to mimic this behavior for the past 20 years, creating the so-called smart polymers (SPs). The characteristic feature that actually makes them smart is their ability to respond to very slight changes in the surrounding environment, such as temperature, pH, light, magnetic or electric eld, ionic factors, and biological molecules. The responses are manifested as changes in one or more of the following: shape, surface characteristics, solubility, formation of an intricate molecular assembly, a sol-to-gel transition, and others (Kumar et al., 2007). The uniqueness of these materials lies not only in the fast macroscopic changes occurring in their structure but also in these transitions being reversible. SPs have very promising applications in the biomedical eld as delivery systems of therapeutic agents, tissue engineering scaffolds, cell culture supports, bioseparation devices, sensors, or actuator systems. Among various SPs, the materials that can sense signals and produce a de nite dynamic response in the form of a change in shape or volume are under active investigation, such as shape-memory polymers (Lendlein et al., 2005), polymer gels (Liu and Calver, 2000; Zriny et al., 2000; Osada and Gong, 1998; Suzuki et al.,

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275 explained in terms of the phenomenological theory (Section 5.2.2) by the procedure proposed by A. N. Frumkin. In the electrode reaction the reacting particles approach the electrode to the smallest possible distance they can reach without adsorption, i.e. to the outer Helmholtz plane. The concentrations of reacting particles at this distance from the electrode, c'Ox and c Red , are given by Eq. (4.3.5) as / zOxFct>2\ Cox = c O x e x p ^ - RT )

The value of the electric potential affecting the activation enthalpy of the electrode reaction is decreased by the difference in the electrical potential between the outer Helmholtz plane and the bulk of the solution, 02> so that the activation energies of the electrode reactions are not given by Eqs (5.2.10) and (5.2.18), but rather by the equations AHC = AH + anF(E - 4>2)

Smart Light Responsive Materials. Edited by Yue Zhao and Tomiki Ikeda Copyright r 2009 John Wiley & Sons, Inc.

As a result of these advances, the server market was born, creating the roots for many later variations, including application servers, clustered servers, NAS, and eventually blade servers..

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Finally, other type of phase separation can help achieving marked macroscopic ampli cation upon crossing a critical condition of demixing In addition to LCST properties, water-soluble polymer can also be made abruptly insoluble upon association with nanoparticles, such as a protein and micelles of surfactants (Piculell and Lindman, 1992) Owing to their importance for industrial products (cosmetic, food, personal care), polymer surfactant demixings have been extensively studied Making these system responsive to light would open a vast range of applications Two classes of phase separation have to be distinguished, namely, seggregative (formation of a surfactant-rich phase and a polymer-rich one, when the two partners have no propensity to bind) and associative separation (demixing of a dense phase containing associates of surfactant and polymer) Here we are interested in the associative separation because photoisomerization could signi cantly affect the association strength.