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The overall Galvani potential difference between the bulk of the semiconductor and the bulk of the electrolyte solution can be separated into three parts: Ar< = Af 0 + A|0 + Al2(j) (4.5.6) where Af$ is the potential difference between the bulk of the semiconductor and the semiconductor-electrolyte interface, A|0 is the potential difference in the compact layer (i.e. between the interface and the outer Helmholtz plane) and A 0 is the potential difference between the outer Helmholtz plane and the bulk of the electrolyte solution. Obviously,

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depicted in Fig. 2.4a have been reported (Gao et al., 2007b). However, the lms of this H-bonded azobenzene polymer (Fig. 2.4f) exhibited dichroic ratio of only 1.2. When in another investigation (Priimagi et al., 2007), commercially available azodye (Disperse Red 1) forming relatively week H-bond with the same polyvinylpyridine (Fig. 2.4h) has been used, relatively high birefringence of 0.035 has been attained. Even higher value of birefringence (0.04, highest value for H-bonded complexes) has been obtained when the same azobenzene derivative was used in combination with polyvinylphenol using the opportunity of another H-bonding (Fig. 2.4h). All this improvement in photoinduced orientation (guest host system of the same dyes and polystyrene (PS) exhibited only birefringence of 0.005) was attributed to the prevention of dye aggregation due to formation of H-bonding [Priimagi et al., 2007). Rather different approach was realized earlier (Gao et al., 2007a), and it is based on intermolecular multiple H-bonding in azobenzene derivative forming an H-bonded main-chain azobenzene polymer (Fig. 2.4e). The latter material showed rather higher dichroic ratio of 5.5. On the contrary, mass transport properties of these last two polymers (discussed later) were vice versa. All these data cannot be analyzed, as different values (birefringence and dichrosim) have been measured; however, it shows that by a variation of H-bond strength, structure of the azobenzene and polymer, signi cant modi cation of optical properties is possible. In contrast to the H-bonded complexes, complexes based on ionic interactions have gained a much greater interest. Such complexes emerged as a multilayer

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Q429345 - BarCodeControl Example | DevExpress Support Center
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